2016
DOI: 10.1021/acsphotonics.5b00499
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Electrodynamic Modeling of Quantum Dot Luminescence in Plasmonic Metamaterials

Abstract: A self-consistent approach is proposed to simulate a coupled system of quantum dots (QDs) and metallic metamaterials. Using a four-level atomic system, an artificial source is introduced to simulate the spontaneous emission process in the QDs. We numerically show that the metamaterials can lead to multifold enhancement and spectral narrowing of photoluminescence from QDs. These results are consistent with recent experimental studies. The proposed method represents an essential step for developing and understan… Show more

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Cited by 21 publications
(8 citation statements)
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“…Since then, the modified SE rate has been observed in various photonic structures, such as microcavities 9 , wisperirng guided cavities 10 , 11 , photonic crystals 12 , 13 , and so on. In recent years, large enhancement of SE have also been reported in theoretically and experimental studies of plasmonic metamaterials 14 , 15 and plasmonic nanostructures 16 23 ; sepcifically, in gap surface plasmon (GSP) structures, the emission rate can exceed 1000 γ 0 , where γ 0 is the SE rate in vacuum, due to the presence of ultrastrong hotspots 18 23 . It is important to note here that these plasmon nanostructures are passive; once fabricated, they do not allow tunability demanded by state-of-the-art nanophotonic devices.…”
Section: Introductionmentioning
confidence: 95%
“…Since then, the modified SE rate has been observed in various photonic structures, such as microcavities 9 , wisperirng guided cavities 10 , 11 , photonic crystals 12 , 13 , and so on. In recent years, large enhancement of SE have also been reported in theoretically and experimental studies of plasmonic metamaterials 14 , 15 and plasmonic nanostructures 16 23 ; sepcifically, in gap surface plasmon (GSP) structures, the emission rate can exceed 1000 γ 0 , where γ 0 is the SE rate in vacuum, due to the presence of ultrastrong hotspots 18 23 . It is important to note here that these plasmon nanostructures are passive; once fabricated, they do not allow tunability demanded by state-of-the-art nanophotonic devices.…”
Section: Introductionmentioning
confidence: 95%
“…Considering a more realistic case, the synchronous of the oscillations and the directionality are limited by the finite size of the metaruface and the pump source [34]. To determine the dimensions of the proposed nanoemitter and to explore the properties of the resonance modes, we employ the FDTD method [40][41][42] to simulate the spectra of the metasurface and grating under normal excitation by a transverse electric (y-polarized) wave. For the grating reflector with periodicity D = 600 nm, the electric dipole mode can be excited and can achieve ~100% around the resonant peak as shown in Fig.…”
Section: Simulation Detailsmentioning
confidence: 99%
“…Both nonlocal and nonlinear effects can be considered using the self-consistent formulations. The multiphysics equations can be numerically solved by employing the FDTD method [23][24][25][26][27], which has been extended to model nonlinear and nonlocal effects in dispersive media.…”
Section: Electromagnetic-hydrodynamic Modelmentioning
confidence: 99%