Electrocatalytic Dinitrogen Reduction to Ammonia Using Easily Reducible N‐Fused Cobalt Porphyrins
Ashwin Ganesan,
Alireza Hajiseyedjavadi,
Pinki Rathi
et al.
Abstract:Single‐site molecular electrocatalysts, especially those that perform catalytic conversion of N2 to NH3 under mild conditions, are highly desirable to derive fundamental structure‐activity relations and as potential alternatives to the current energy‐consuming Haber‐Bosch ammonia production process. Combining theoretical calculations with experimental evidence, it has been shown that easily reducible cobalt porphyrins catalyze the six‐electron, six‐proton reduction of dinitrogen to NH3 at neutral pH and under … Show more
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