Abstract:Epitaxial thin films of optimally doped, underdoped, and Zn-doped YBa 2 Cu 3 O 7−␦ ͑YBCO͒ were grown on single crystal ͑001͒ Nb: SrTiO 3 substrates by pulsed laser deposition ͑PLD͒ and the electrical properties of the corresponding interface junctions were examined. The growth conditions were optimized in each case to get the appropriate crystalline quality of the films as well as the desired normal state and superconducting properties. The films or heterointerfaces were characterized by x-ray diffraction, Rut… Show more
“…Interfacial couplings in such heterostructures can potentially present a wide range of emergent phenomena. 16 Indeed, a variety of fascinating properties has been evidenced in YBCO-based junctions, [17][18][19][20][21] rendering the BFO/YBCO heterostructure an excellent candidate in the search for novel properties in low dimensions.…”
We report the synthesis and characterization of an epitaxial heterostructure composed of multiferroic BiFeO 3 and superconducting YBa 2 Cu 3 O 7−␦ thin films grown on ͑001͒ SrTiO 3 . Both the superconductivity of YBa 2 Cu 3 O 7−␦ and the ferroelectricity of BiFeO 3 are retained in the heterostructure. Current density-electric field characteristics measured from 30 to 170 K suggest a Schottky-emission-like transport at the BiFeO 3 / YBa 2 Cu 3 O 7−␦ interface. Furthermore, the temperature dependence of the barrier height shows an anomalous enhancement at T C , indicating an intimate coupling between the multiferroic and the superconducting layers.
“…Interfacial couplings in such heterostructures can potentially present a wide range of emergent phenomena. 16 Indeed, a variety of fascinating properties has been evidenced in YBCO-based junctions, [17][18][19][20][21] rendering the BFO/YBCO heterostructure an excellent candidate in the search for novel properties in low dimensions.…”
We report the synthesis and characterization of an epitaxial heterostructure composed of multiferroic BiFeO 3 and superconducting YBa 2 Cu 3 O 7−␦ thin films grown on ͑001͒ SrTiO 3 . Both the superconductivity of YBa 2 Cu 3 O 7−␦ and the ferroelectricity of BiFeO 3 are retained in the heterostructure. Current density-electric field characteristics measured from 30 to 170 K suggest a Schottky-emission-like transport at the BiFeO 3 / YBa 2 Cu 3 O 7−␦ interface. Furthermore, the temperature dependence of the barrier height shows an anomalous enhancement at T C , indicating an intimate coupling between the multiferroic and the superconducting layers.
“…[9][10][11][12] Furthermore, TMO exhibits distinct magnetic phases in various temperature regimes: the collinear spin order of Mn ions sets in at a Neel temperature T N of 41 K; the ferroelectric phase emerges in the bc-spiral spin state below 28 K, and concurrently the magnetic and the polarization vectors orientate along the b and the c axis, respectively; finally, a phase transition at about 7 K appears as a result of the magnetic ordering of the Tb sublattice. 4 As the first step towards the oxide electronics, a wide range of transition metal oxides are exploited in various device concepts, such as Schottky-like junctions, [13][14][15][16] field-effect transistors, 17,18 a Email: tomwu@ntu.edu.sg; rmwang@buaa.edu.cn 2158-3226/2011/1(4)/042129/11 C Author(s) 2011 1, 042129-1 and p-n junctions, [19][20][21][22][23] which are the building blocks in conventional semiconductor electronics. 24 Among them, two-terminal junctions are often considered as the most fundamental one due to their ubiquitous presence in many devices with higher complexity.…”
We report the fabrication and characterizations of oxide heterojunctions composed of TbMnO3 thin films grown on conducting Nb:SrTiO3 substrates. The heterojunctions exhibit rich rectifying characteristics, depending on not only the measurement temperature but also the growth temperature: at 300 K, good rectification appears in both samples; at lower temperatures, the rectification is much smaller in the sample grown at 700 °C, whereas it exhibits a reversed bias dependence and reaches ∼5000 in the sample grown at 780 °C. Regarding to the transport mechanism, the conduction appears to be Schottky-emission-like at high temperatures in both junctions, indicating well-defined band alignment at interface; on the other hand, the space-charge-limited mechanism dictates the low temperature transport. Furthermore, the temperature and frequency dependent capacitance-loss data suggest that the transport dynamics is associated with multiple thermally activated relaxation processes. Finally, transmission electron microscopy studies shed light on the crystalline quality of the junction interfaces, which is believed to dictate the corresponding transport properties
“…Indeed, a variety of fascinating properties have been evidenced in YBCO-based junctions. [171][172][173][174][175] Epitaxial growth of BFO/YBCO heterostructure can be realized due to the compatible lattice structure in the two materials with a lattice mismatch of $3%. Interfacial couplings in such heterostructures may drastically upset the delicate balance of the competing interactions among charges, spins, orbitals, and lattice, which can potentially present a wide range of emergent phenomena.…”
Multiferroic materials promise a tantalizing perspective of novel applications in next-generation electronic, memory, and energy harvesting technologies, and at the same time they also represent a grand scientific challenge on understanding complex solid state systems with strong correlations between multiple degrees of freedom. In this review, we highlight the opportunities and obstacles in growing multiferroic thin films with chemical and structural integrity and integrating them in functional devices. Besides the magnetoelectric effect, multiferroics exhibit excellent resistant switching and photovoltaic properties, and there are plenty opportunities for them to integrate with other ferromagnetic and superconducting materials. The challenges include, but not limited, defect-related leakage in thin films, weak magnetism, and poor control on interface coupling. Although our focuses are Bi-based perovskites and rare earth manganites, the insights are also applicable to other multiferroic materials. We will also review some examples of multiferroic applications in spintronics, memory, and photovoltaic devices.
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