Abstract:Photocatalytic hydrogen peroxide (H2O2) generation represents a promising approach for artificial photosynthesis. However, the sluggish half-reaction of water oxidation significantly limits the efficiency of H2O2 generation. A substitutional reaction of oxidation with accelerated kinetics to produce value-added chemicals holds promise to tackle this challenge. Here, a benzylamine oxidation with more favorable thermodynamics is employed as the half-reaction to couple with H2O2 generation in water by using defec… Show more
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