Efficient NADH Regeneration without Electron Mediator toward Enzymatic CO2 Reduction Enabled by a Lawn-like TP-COFs/Ti3C2Tx (MXene) Photocatalyst
Ping Wei,
Jinfeng Dong,
Xingyue Gao
et al.
Abstract:Photocatalytic nicotinamide adenine dinucleotide (NADH) regeneration coupled with enzymatic CO 2 reduction holds significance for global sustainable development. In this work, acrylonitrile-linked covalent organic frameworks (COFs) loaded on NH 2 −Ti 3 C 2 T x (MXene) forms a lawn-like TP-COFs/Ti 3 C 2 T x (TCM) photocatalyst for NADH regeneration. The optimum photocatalyst TCM-15% achieves a 95% NADH regeneration yield within 30 min. More importantly, the TCM-15% obtains 46% NADH regeneration yield without an… Show more
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