Efficient CO2 fixation with acetophenone on Ag-CeO2 electrocatalyst by a double activation strategy

Guan, Anxiang; Quan, Yueli; Chen, Yangshen; Liu, Zhengzheng; Zhang, Junbo; Kan, Miao; Zhang, Quan; Huang, Haoliang; Qian, Linping; Zhang, Linjuan; Zheng, Gengfeng

doi:10.1016/s1872-2067(22)64116-0

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Electrocarboxylation Of Aromatic Ketones1

Reductive Electrochemical Organic Transformations With Co2 A...1

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2023

2024

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Cited by 7 publications

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Section: Electrocarboxylation Of Aromatic Ketonesmentioning

confidence: 99%

“…Guan et al showed that double activation by the Ag-CeO 2 NW catalyst led to the electrocarboxylation of acetophenone with CO 2 to form 2-phenyllactic acid. 70 The dual-site Ag-CeO 2 NWs exhibited the ability to activate both CO 2 and acetophenone concurrently through cathodic activation, resulting in the synergistic generation of CO 2 ˙ − and ketyl radical anions, thus favoring the electrocarboxylation process. Notably, the desired 2-phenyllactic acid product was produced with a maximum FE = 91% at −1.8 V Ag/AgI (entry 9 in Table 1).…”

Section: Reductive Electrochemical Organic Transformations With Co2 A...mentioning

confidence: 99%

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