2011
DOI: 10.1364/josab.28.001680
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Efficient bidirectional optical harmonics generation in three-dimensional photonic crystals

Abstract: Noncollinear generation of second and third harmonics in three-dimensional photonic crystals of artificial opals is experimentally realized and interpreted in terms of nonlinear diffraction. A factor-of-two enhancement of second-and third-harmonic generation intensity in diffraction maxima directions is observed due to effective phase matching provided by photonic crystal periodicity. Bidirectional diffraction of third harmonics at crystallographic planes ð111Þ and ð 1 11Þ is observed. The broadening of nonspe… Show more

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Cited by 7 publications
(3 citation statements)
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“…This led to an inverse opal showing second harmonic generation (Figure b). These nonlinear optical inverse opals will be investigated further as the anomalous dispersion in such structures is believed to cause phase matching effects, which considerably boost the efficiency of nonlinear scattering effects. , …”
Section: Resultsmentioning
confidence: 99%
“…This led to an inverse opal showing second harmonic generation (Figure b). These nonlinear optical inverse opals will be investigated further as the anomalous dispersion in such structures is believed to cause phase matching effects, which considerably boost the efficiency of nonlinear scattering effects. , …”
Section: Resultsmentioning
confidence: 99%
“…The effect of the second harmonic generation looks unusual for a non-crystalline amorphous material of SiO 2 glob- ules. The reported observation of the effect is related to the situation of the opal matrix filled with immersion [7], and the mechanism is explained with account for the local breaking of the inversion symmetry at the surface of each spherical particle [8]. However, the nonlinear polarization at the second harmonic frequency can appear owing to the interference of an extremely high-power pulse with a seed radiation in the material [9].…”
Section: Introductionmentioning
confidence: 99%
“…Nonlinear diffraction was originally reported for second-harmonic generation (SHG) in systems with periodic spatial modulation of the quadratic susceptibility χ (2) . The nonlinear diffraction of SHG and third-harmonic generation (THG) was further demonstrated for various periodic systems including 2D and 3D nonlinear photonic crystals. , In these systems, second or third harmonics were generated efficiently as the nonlinear Bragg law was fulfilled at the quasi-phase matching condition. Diffraction is also actively studied in metasurfaces, 2D arrays of subwavelength nanoresonators, which allow one to manipulate the phase, amplitude, and polarization of transmitted or reflected light by engineering the constituent elements (i.e., meta-atoms) .…”
mentioning
confidence: 99%