Herein, various nickel cobalt oxide nanostructures with different Ni concentrations are prepared via hydrothermal route and then calcination process for electrochemical supercapacitor as well as nonenzymatic glucose biosensor. The electrode synthesized on carbon cloth using Ni 0.9 Co 2.1 O 4 nanosheet-like morphology showed a maximum 516.51 F g −1 speci c capacitance at 10 mV s −1 scan rate and the cyclic stability of 87.7% over 2000 GCD cycles. The electrode prepared with Ni 0.3 Co 2.7 O 4 on CC offered a linear response from 0 to 0.3 mM glucose concentration and exhibited a maximum of 759.5 µA mM −1 cm −2 glucose sensitivity.