Abstract:We present a high-performance functional perfect absorber in a wide range of terahertz (THz) wave based on a hybrid structure of graphene and vanadium dioxide (VO2) resonators. Dynamically electrical and thermal tunable absorption is achieved due to the management on the resonant properties via the external surroundings. Multifunctional manipulations can be further realized within such absorber platform. For instance, a wide-frequency terahertz perfect absorber with the operation frequency range covering from … Show more
“…In the THz and MW regions, the dielectric constants of VO 2 can be described using the Drude model 45 , 46 : where ε ∞ = 12 is dielectric permittivity at the infinite frequency, is the plasma frequency of VO 2 that dependent on conductivity, = 5.75 ×10 13 rad· s −1 is the collision frequency, = 3 ×10 5 S· m −1 , = 1.5 ×10 15 rad· s −1 , is the conductivity of VO 2 (Fig. 4d and Supplementary Fig.…”
Optical materials capable of dynamically manipulating electromagnetic waves are an emerging field in memories, optical modulators, and thermal management. Recently, their multispectral design preliminarily attracts much attention, aiming to enhance their efficiency and integration of functionalities. However, the multispectral manipulation based on these materials is challenging due to their ubiquitous wavelength dependence restricting their capacity to narrow wavelengths. In this article, we cascade multiple tunable optical cavities with selective-transparent layers, enabling a universal approach to overcoming wavelength dependence and establishing a multispectral platform with highly integrated functions. Based on it, we demonstrate the multispectral (ranging from 400 nm to 3 cm), fast response speed (0.9 s), and reversible manipulation based on a typical phase change material, vanadium dioxide. Our platform involves tandem VO2-based Fabry–Pérot (F-P) cavities enabling the customization of optical responses at target bands independently. It can achieve broadband color-changing capacity in the visible region (a shift of ~60 nm in resonant wavelength) and is capable of freely switching between three typical optical models (transmittance, reflectance, and absorptance) in the infrared to microwave regions with drastic amplitude tunability exceeding 0.7. This work represents a state-of-art advance in multispectral optics and material science, providing a critical approach for expanding the multispectral manipulation ability of optical systems.
“…In the THz and MW regions, the dielectric constants of VO 2 can be described using the Drude model 45 , 46 : where ε ∞ = 12 is dielectric permittivity at the infinite frequency, is the plasma frequency of VO 2 that dependent on conductivity, = 5.75 ×10 13 rad· s −1 is the collision frequency, = 3 ×10 5 S· m −1 , = 1.5 ×10 15 rad· s −1 , is the conductivity of VO 2 (Fig. 4d and Supplementary Fig.…”
Optical materials capable of dynamically manipulating electromagnetic waves are an emerging field in memories, optical modulators, and thermal management. Recently, their multispectral design preliminarily attracts much attention, aiming to enhance their efficiency and integration of functionalities. However, the multispectral manipulation based on these materials is challenging due to their ubiquitous wavelength dependence restricting their capacity to narrow wavelengths. In this article, we cascade multiple tunable optical cavities with selective-transparent layers, enabling a universal approach to overcoming wavelength dependence and establishing a multispectral platform with highly integrated functions. Based on it, we demonstrate the multispectral (ranging from 400 nm to 3 cm), fast response speed (0.9 s), and reversible manipulation based on a typical phase change material, vanadium dioxide. Our platform involves tandem VO2-based Fabry–Pérot (F-P) cavities enabling the customization of optical responses at target bands independently. It can achieve broadband color-changing capacity in the visible region (a shift of ~60 nm in resonant wavelength) and is capable of freely switching between three typical optical models (transmittance, reflectance, and absorptance) in the infrared to microwave regions with drastic amplitude tunability exceeding 0.7. This work represents a state-of-art advance in multispectral optics and material science, providing a critical approach for expanding the multispectral manipulation ability of optical systems.
“…[18,19] Similarly, studies on aerogels composed of phase change materials exhibited switching behavior, but with a more limited tuning range. [13,14] For example, Chang et al reported RL tuned from −17 to −54 dB, corresponding to a modulation in absorption in the range from 98% to ≈100%. [28] In addition, the tuning often covered a relatively narrow band with frequencies mostly located in the microwave range instead of in the THz range.…”
“…Switchable materials that can modulate the absorption or transmission of THz signals are useful for intelligent calibration targets, dynamic attenuators for THz optical circuits, and effective modulators for electromagnetic interference, as demonstrated by multiple simulation results. [13][14][15] Only a few materials have shown decent tunability in the THz range, [13,14,[16][17][18][19] despite significant research progress in electromagnetic absorbers. [20][21][22][23][24][25][26] Several of these systems focused on modulating THz properties via reflection rather than absorption, and often with limited tuning range.…”
Terahertz (THz) technologies provide opportunities ranging from calibration targets for satellites and telescopes to communication devices and biomedical imaging systems. A main component will be broadband THz absorbers with switchability. However, optically switchable materials in THz are scarce and their modulation is mostly available at narrow bandwidths. Realizing materials with large and broadband modulation in absorption or transmission forms a critical challenge. This study demonstrates that conducting polymer‐cellulose aerogels can provide modulation of broadband THz light with large modulation range from ≈ 13% to 91% absolute transmission, while maintaining specular reflection loss < −30 dB. The exceptional THz modulation is associated with the anomalous optical conductivity peak of conducting polymers, which enhances the absorption in its oxidized state. The study also demonstrates the possibility to reduce the surface hydrophilicity by simple chemical modifications, and shows that broadband absorption of the aerogels at optical frequencies enables de‐frosting by solar‐induced heating. These low‐cost, aqueous solution‐processable, sustainable, and bio‐friendly aerogels may find use in next‐generation intelligent THz devices.
“…[32] Hence, in-depth studies on the versatile or frequency reconfigurable MS enter a new boom by combining metallic resonators and tunable materials. Considerable methods of regulation include but are not limited to temperature, [33,34] gravity field, [35] illumination, [36,37] and electric field. [38] For instance, Singh et al experimentally demonstrated and compared the thermal tuning of the fundamental inductive-capacitive resonance, where metals and superconductors are discussed, to active MS resonance tuning.…”
Section: Introductionmentioning
confidence: 99%
“…[ 32 ] Hence, in‐depth studies on the versatile or frequency reconfigurable MS enter a new boom by combining metallic resonators and tunable materials. Considerable methods of regulation include but are not limited to temperature, [ 33,34 ] gravity field, [ 35 ] illumination, [ 36,37 ] and electric field. [ 38 ] For instance, Singh et al.…”
With the tunability of the nematic liquid crystal (NLC), a broadband frequency reconfigurable and versatile metastructure (MS) is proposed and theoretically investigated in this paper, combining circular‐to‐linear (CTL) polarization conversion (PC) and circular‐to‐circular (CTC) PC simultaneously. The MS is composed of two via‐coupled modules, which can respond differently to the incident waves. Each module is connected utilizing a metal via a column, thus exceedingly enhancing the energy transmission and reducing the loss when transmitting. When the applied bias voltage (Vbias) is 0 V, the NCL molecules follow the initial orientation. The MS converts the incident right circular polarized (RCP) waves into linear polarized (LP) waves within 8.11–9.95 gigahertz (GHz) with a relative bandwidth of 20.38% and achieves the PC of left circular polarized (LCP) into RCP waves. As the Vbias reaches 20 V, the original operating interval reconfigures and shifts overall toward a lower frequency. The bandwidth of CTL is 7.66–9.02 GHz, and the CTC PC is broadened to 20.20%. Meanwhile, the structure justification is verified, and the inducing mechanism of PC is expounded. Possessing the merits of versatile collaborative processing and wide operating bands, such an MS is promising to be a polarization‐controlled application candidate and enrich multifunctional designs.
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