Effective tracer-test design requires that the likely results be predicted in advance of test initiation to ensure tracer-test success. EHTD-predicted breakthrough curves (BTCs) for various hydrological conditions were compared with measured BTCs obtained from actual tracer tests. The hydrological conditions for the tracer tests ranged from flowing streams to porous-media systems. Tracer tests evaluated included flowing streams tracer tests conducted in small and large surface-water streams, a karst solution conduit, and a glacial-meltwater stream and porous-media systems conducted as natural-gradient, forced-gradient, injection-withdrawal, and recirculation tracer tests. Comparisons between the actual tracer tests and the predicted results showed that tracer breakthrough, hydraulic characteristics, and sample-collection frequency may be forecasted sufficiently well in most instances as to facilitate good tracer-test design. Comparisons were generally improved by including tracer decay and/or retardation in the simulations. Inclusion of tracer decay in the simulations also tended to require an increase in set average tracer concentration to facilitate matching peak concentrations in the measured BTCs, however. Both nonreactive tracer and reactive tracer predictions produced recommended sample-collection frequencies that would adequately define the actual BTCs, but estimated tracer-mass estimates were less precise.