Dual chemifunctional tin(IV) oxide/nanoperforated graphene interlayer as a polysulfide adsorbent for use in high-performance lithium–sulfur batteries

Lee, Junho; Hwang, Sang Yeop; Oh, Byeong Il; Jeon, Young Gyu; Jung, Nae Yeon; Ahn, Wook; Lim, Hyung-Kyu; Kim, Hyun-Kyung

doi:10.1016/j.cej.2023.147996

Chemical Engineering Journal

2024

DOI: 10.1016/j.cej.2023.147996

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Dual chemifunctional tin(IV) oxide/nanoperforated graphene interlayer as a polysulfide adsorbent for use in high-performance lithium–sulfur batteries

Junho Lee,

Sang Yeop Hwang,

Byeong Il Oh

et al.

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Pristine MOF Materials for Separator Application in Lithium–Sulfur Battery

Cheng,

Lian,

Zhang

et al. 2024

Advanced Science

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Lithium–sulfur (Li–S) batteries have attracted significant attention in the realm of electronic energy storage and conversion owing to their remarkable theoretical energy density and cost‐effectiveness. However, Li–S batteries continue to face significant challenges, primarily the severe polysulfides shuttle effect and sluggish sulfur redox kinetics, which are inherent obstacles to their practical application. Metal‐organic frameworks (MOFs), known for their porous structure, high adsorption capacity, structural flexibility, and easy synthesis, have emerged as ideal materials for separator modification. Efficient polysulfides interception/conversion ability and rapid lithium‐ion conduction enabled by MOFs modified layers are demonstrated in Li–S batteries. In this perspective, the objective is to present an overview of recent advancements in utilizing pristine MOF materials as modification layers for separators in Li–S batteries. The mechanisms behind the enhanced electrochemical performance resulting from each design strategy are explained. The viewpoints and crucial challenges requiring resolution are also concluded for pristine MOFs separator in Li–S batteries. Moreover, some promising materials and concepts based on MOFs are proposed to enhance electrochemical performance and investigate polysulfides adsorption/conversion mechanisms. These efforts are expected to contribute to the future advancement of MOFs in advanced Li–S batteries.

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Pristine MOF Materials for Separator Application in Lithium–Sulfur Battery

Cheng,

Lian,

Zhang

et al. 2024

Advanced Science

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Dual chemifunctional tin(IV) oxide/nanoperforated graphene interlayer as a polysulfide adsorbent for use in high-performance lithium–sulfur batteries

Cited by 1 publication

References 73 publications

Pristine MOF Materials for Separator Application in Lithium–Sulfur Battery

Pristine MOF Materials for Separator Application in Lithium–Sulfur Battery

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