Does the ionic distribution in the electrical double layer modify second harmonic scattering?
Bingxin Chu,
Sylvie Roke,
Arianna Marchioro
Abstract:Surface-specific nonlinear optical techniques are ideally suited to investigate the complex structure of aqueous interfaces. For colloidal particles dispersed in aqueous solutions, interfacial properties can be retrieved with angle-resolved second harmonic scattering (AR-SHS). The mathematical framework of AR-SHS does not require a priori knowledge on the electrostatic distribution in the first few nanometers close to the interface, therefore allowing us to formulate a molecular-level description of the electr… Show more
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