Direct Solution-calcination synthesis of residual Li-free layered cathode materials for Li-ion batteries

Choi, Yoo Jung; Kim, You Jin; Kim, Suji; Kim, Ga Yoon; Ryu, Won‐Hee

doi:10.1016/j.apsusc.2023.157444

Applied Surface Science

2023

DOI: 10.1016/j.apsusc.2023.157444

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Direct Solution-calcination synthesis of residual Li-free layered cathode materials for Li-ion batteries

Yoo Jung Choi

You Jin Kim

Suji Kim

et al.

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Cited by 3 publications

References 59 publications

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In Situ Gas Analysis by Differential Electrochemical Mass Spectrometry for Advanced Rechargeable Batteries: A Review

Kim,

Kim

et al. 2023

Advanced Energy Materials

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Lithium‐ion batteries (LIBs) and beyond‐LIB systems exhibit properties that are determined by electrochemical reactions occurring in their four essential components—the cathode, anode, electrolyte, and separator. Advanced analytical methods such as differential electrochemical mass spectrometry (DEMS) can assist in understanding the electrochemical behavior, which can help in advancing battery technologies. Recent studies have shown that the DEMS‐enabled real‐time gas analysis of electrochemical reactions can provide valuable information on aspects such as gaseous reactants or (side) products, which cannot be obtained appropriately through other characterization techniques. This review aims to provide a comprehensive overview of the latest developments and advancements in the use of DEMS as a rapid, operando gas‐monitoring method for advanced rechargeable battery systems. Moreover, the significance of DEMS in current and future battery development is also discussed and insights are provided into the various battery chemistries that can benefit from DEMS applications. This review is intended to help readers understand the potential of DEMS to drive innovation in the battery industry.

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In Situ Gas Analysis by Differential Electrochemical Mass Spectrometry for Advanced Rechargeable Batteries: A Review

Kim,

Kim

et al. 2023

Advanced Energy Materials

Self Cite

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Asymmetrical Functionalization of Polarizable Interface Restructuring Molecules for Rapid and Longer Operative Lithium Metal Batteries

Son,

Kim,

Jun

et al. 2024

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Lithium metal batteries (LMBs) have been recognized as high‐energy storage alternatives; however, problematic surface reactions due to dendritic Li growth are major obstacles to their widespread utilization. Herein, a 3‐mercapto‐1‐propanesulfonic acid sodium salt (MPS) with asymmetrically functionalized thiol and sulfonate groups as polarizable interface‐restructuring molecules is proposed to achieve rapid and longer‐operating LMBs. Under a harsh condition of 5 mA cm−2, Li–Li symmetric cells employing MPS can be cycled over 1200 cycles, outperforming those employing other molecules symmetrically functionalized by thiol or sulfonate groups. The improved performance of the Li|V2O5 full cell is demonstrated by introducing MPS additives. MPS additives offer advantages by flattening the surface, reconfiguring Li nucleation and growth along the stable (110) plane, and forming a durable and conductive solid–electrolyte interface layer (SEI). This study suggests an effective way to develop a new class of electrolyte additives for LMBs by controlling engineering factors, such as functional groups and polarizable properties.

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Engineering aspects of sodium-ion battery: An alternative energy device for Lithium-ion batteries

Wanison,

Syahputra,

Kammuang-lue

et al. 2024

Journal of Energy Storage

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Direct Solution-calcination synthesis of residual Li-free layered cathode materials for Li-ion batteries

Cited by 3 publications

References 59 publications

In Situ Gas Analysis by Differential Electrochemical Mass Spectrometry for Advanced Rechargeable Batteries: A Review

In Situ Gas Analysis by Differential Electrochemical Mass Spectrometry for Advanced Rechargeable Batteries: A Review

Asymmetrical Functionalization of Polarizable Interface Restructuring Molecules for Rapid and Longer Operative Lithium Metal Batteries

Engineering aspects of sodium-ion battery: An alternative energy device for Lithium-ion batteries

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