2023
DOI: 10.1140/epjd/s10053-023-00759-6
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Dipole instability in molecules irradiated by XUV pulses

D. Hughes,
D. Dundas,
P. M. Dinh
et al.

Abstract: We study the response of small covalent molecules to XUV laser pulses. The theoretical description relies on a real-time and real-space Time-Dependent Density Functional Theory (TDDFT) approach at the level of the local density approximation complemented by an efficient self-interaction correction. We observe the development of a dipole instability well after the laser pulse has died out. We find that this instability mechanism is robust with respect to ionic motion, to a wide variety of laser characteristics… Show more

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