Abstract:We present for the first time a SESAM-modelocked thin-disk laser (TDL) that incorporates two gain materials with different emission spectra in a single TDL resonator. The two gain media used in this experiment are the sesquioxide materials Yb:Lu 2 O 3 and Yb:Sc 2 O 3 , which have their spectral emission peak displaced by ≈7 nm. We can benefit from a combined gain bandwidth that is wider than the one provided by a single gain material alone and still conserve the excellent thermal properties of each disk. In these first proof-of-principle experiments we demonstrate pulse durations shorter than previously achieved with the single gain material Yb:Lu 2 O 3 . The oscillator generates pulses as short as 103 fs at a repetition rate of 41.7 MHz and a center wavelength of around 1038 nm, with an average output power of 1.4 W. A different cavity layout provides pulses with a duration of 124 fs at an output power of 8.6 W. This dual-gain approach should allow for further power scaling of TDLs and these first results prove this method to be a promising new way to combine the record output-power performance of modelocked TDLs with short pulse durations in the sub-100 fs regime. Matuschek, and J. Aus der Au, "Semiconductor saturable absorber mirrors (SESAMs) for femtosecond to nanosecond pulse generation in solid-state lasers," IEEE J. Sel. Top. Quantum Electron. 2(3), 435-453 (1996). 2. A. Giesen, H. Hügel, A. Voss, K. Wittig, U. Brauch, and H. Opower, "Scalable concept for diode-pumped highpower solid-state lasers," Appl. Phys. B 58(5), 365-372 (1994). Published in Optics Express, 22, issue 16, 18979-18986, 2014 which should be used for any reference to this work 1 Stolow, U. Thumm, and M. J. J. Vrakking, "What will it take to observe processes in 'real time'?" Nat. Photonics 8(3), 162-166 (2014