Abstract:Adhesives with superior toughness and self-healing properties are critical for the practical application of energetic composite materials (ECMs). However, most self-healing polymers exhibit low creep resistance and toughness, which makes simultaneous optimization a challenge. To overcome this, we introduced asymmetric alicyclic and bent biphenyl ring structures into the hard domain units of soft polymers, which resulted in adhesives with robust mechanical properties. The synergistic effect of dynamic disulfide… Show more
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