“…Organic light-emitting diodes (OLEDs) have achieved great progress in the past 3 decades because of the potential applications in flat-panel display and solid-state lighting. − In OLED devices, spin-uncorrelated hole and electron carriers are injected from the anode and cathode, respectively; then, they recombine to form excitons with either spin-singlet or -triplet character in a ratio of 1:3 following the spin statistics. , Thus, to develop high-efficiency OLEDs, it is critical to harness both the singlet and triplet excitons for light emission . At present, both singlet harvesting mechanisms (e.g., thermally activated delayed fluorescence, TADF) − and triplet harvesting mechanisms (e.g., phosphorescence) − have been proposed to utilize all electrically generated excitons, and the ideal charge-to-photon internal quantum efficiency can reach 100%.…”