The ORCID identification number(s) for the author(s) of this article can be found under https://doi.org/10.1002/adom.201901092.
Electric Bias-Induced ModulationHybrid perovskites (HPs), particularly methylammonium lead iodide (CH 3 NH 3 PbI 3 , hereafter MAPbI 3 ), have attracted enormous attention owing to their outstanding optoelectronic properties, such as tunable bandgap in the visible range, [1,2] long diffusion length, [3,4] superb optical absorption, [5] small exciton binding energy, [6] high ambipolar charge mobility, [7,8] and even ferroelectric polarization. [9] The solution-processed perovskite solar cells exhibit photovoltaic power conversion efficiency over 23%. [10][11][12][13] In addition to photovoltaic applications, HPs have also been exploited for light-emitting diodes, [14,15] lasing