The great Cambro-Ordovician sandstone succession of northern Gondwana is one of the most voluminous siliciclastic deposits on Earth. Its deposition took place following the Neoproterozoic Pan-African Orogeny and the consolidation of Gondwana, a crucial episode in Earth history. Its provenance is of great importance for reconstructing palaeogeographic and tectonic settings and determining sediment dispersal patterns. In Israel and its environs, Palaeozoic sandstones overlie the juvenile Neoproterozoic basement of the Arabian-Nubian Shield. These basement rocks were considered as an important sediment source to the Cambro-Ordovician succession. However, recent studies established that a dominant portion of detrital zircons in the succession was derived from Archean-Proterozoic remobilized terranes, suggesting transportation distances of thousands of kilometres beyond the Arabian-Nubian Shield, and thus question the provenance of other, less weatheringresistant constituents, which were not necessarily derived from the same localities. Feldspars and clays were separated from 13 samples and analyzed for mineralogical and geochemical compositions, strontium, neodymium and lead isotopes, in order to further constrain the provenance of the Cambro-Ordovician succession of northern Gondwana. Detrital feldspars have eNd values significantly different from feldspars of the Arabian-Nubian Shield, ranging from À8 to À14, with model ages of 950 to 1750 Ma, more radiogenic lead compositions, and l ( 238 U/ 204 Pb) values ranging from 9Á8 to 10Á26. Clays are dominated by illite, smectite and kaolinite, with eNd values ranging between À14 and À9, with 87 Sr/ 86 Sr ratios up to 0Á757. These findings point to a significant contribution of remote ancient terranes from outside the Arabian-Nubian Shield to the Cambro-Ordovician sandstone of northern Gondwana. The possible sources for these sediments are the Saharan Metacraton and the southern regions of the East African Orogen.