“…Semiconductor nanowires (NWs), exhibiting the intrinsic quantum-confined 1D structure, have been intensively studied as building blocks for the fabrication of nanoelectronics and photonic devices. [19][20][21][22][23][24][25] Significantly, the electrical and optical properties of NWs can be effectively tuned by controlling the sizes, shapes, and compositions, providing a viable route for tailoring light-matter interaction and achieving the generation, amplification, propagation, and modulation of light on the nanoscale. [8,25,26] Owing to the high carrier mobility, narrow bandgap, tunable light absorption, strong spin-orbit interaction, and considerable subwavelength size effect at room temperature, III-Sb NWs have attracted research attention in the fields of electronics, optoelectronics, and spintronics in the past decades.…”