2018
DOI: 10.1103/physrevapplied.10.064045
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Density and T1 of Surface and Bulk Spins in Diamond in High Magnetic Field Gradients

Abstract: We report on surface and bulk spin density measurements of diamond, using ultra-sensitive magnetic force microscopy with magnetic field gradients up to 0.5 T/µm. At temperatures between 25 and 800 mK, we measure the shifts in the resonance frequency and quality factor of a cantilever with a micromagnet attached to it. A recently developed theoretical analysis allows us to extract a surface spin density of 0.072 spins/nm 2 and a bulk spin density of 0.4 ppm from this data. In addition, we find an increase of th… Show more

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Cited by 6 publications
(2 citation statements)
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“…The bounded range of 0.01 − 0.1/nm 2 is consistent with the densities extracted by various different methods in Refs. [6,49,64].…”
Section: Supplemental Note 2: Surface Spin Density Estimatementioning
confidence: 99%
“…The bounded range of 0.01 − 0.1/nm 2 is consistent with the densities extracted by various different methods in Refs. [6,49,64].…”
Section: Supplemental Note 2: Surface Spin Density Estimatementioning
confidence: 99%
“…A diamond of 230 nm radius contains ∼ 10 9 carbon atoms, which indicates that even for 13 C concentrations as low as 10 −6 % the diamond will contain ∼ 10 3 nuclear spins. On the other hand, the most optimistic estimates for the dangling bond density on the surface of diamond are on the order of 10 −2 dangling bonds per nm 2 (estimated for single crystal bulk diamond grown under optimal conditions) [49], which amounts to a total of 10 3 electron spins on a 230 nm diamond. All in all, one could expect that such a diamond will have a magnetic moment of…”
Section: Constant Homogeneous Forcesmentioning
confidence: 99%