Degradation of amoxicillin from water by ultrasound-zero-valent iron activated sodium persulfate

Sun, Xianke; Qin, Yanxin; Zhou, Wen

doi:10.1016/j.seppur.2021.119080

Cited by 40 publications

(10 citation statements)

References 36 publications

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“…and 428 were present compared with the blank control. Combined with previous studies(Sun et al 2021), the possible degradation pathways of AMX were speculated as shown in FigureS7. The degradation of AMX was a reaction process dominated by the attack of •OH and SO 4 • À .…”

mentioning

confidence: 74%

“…A variety of techniques have been studied to remove AMX from water, such as adsorption (Kerkez-Kuyumcu et al 2016), nanofiltration (Karimnezhad et al 2020), photocatalytic degradation (Moreira et al 2016) and advanced oxidation process (AOP) (Sepyani et al 2018;Sun et al 2021). In contrast, AOP based on sulfate radical (SO 4 • À ) has attracted the most attention due to its high efficiency and wide range of applications (Matzek & Carter 2016).…”

Section: Introductionmentioning

confidence: 99%

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Hydrothermal synthesis of magnetic nano-CoFe2O4 catalyst and its enhanced degradation of amoxicillin by activated permonosulfate

Wang²,

Zhang

et al. 2021

Water Science and Technology

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Advanced oxidation process (AOP) has attracted widespread attention because it can effectively remove antibiotics in water, but its practical engineering application is limited by the problems of the low efficiency and difficult recovery of the catalyst. In the study, nano-spinel CoFe2O4 was prepared by hydrothermal method and served as the peroxymonosulfate (PMS) catalyst to degrade antibiotic amoxicillin (AMX). The reaction parameters such as CoFe2O4 dosage, AMX concentration, and initial pH value were also optimized. The reaction mechanism was proposed through free radical capture experiment and possible degradation pathway analysis. In addition, the magnetic recovery performance and stability of the catalyst were evaluated. Results showed that 85.5% of AMX could be removed within 90 min at optimal conditions. Sulfate radicals and hydroxyl radicals were the active species for AMX degradation. Moreover, the catalyst showed excellent magnetism and stability in the cycle experiment, which has great potential in the AOP treatment of antibiotic polluted wastewater.

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mentioning

confidence: 74%

Section: Introductionmentioning

confidence: 99%

Hydrothermal synthesis of magnetic nano-CoFe2O4 catalyst and its enhanced degradation of amoxicillin by activated permonosulfate

Wang²,

Zhang

et al. 2021

Water Science and Technology

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“…Previous reports indicate that the environmental concentrations of amoxicillin are typically low in raw sewage, which can vary from several ng L −1 to µg L −1 [1,9,12,13], except some rare cases showed mg L −1 levels [12]. The infrequent detection of amoxicillin may be explained by a short retention time of amoxicillin in the environment due to the highly reactive β-lactam ring, which can be broken under environmental conditions and transformed into different products [4,6,[9][10][11]14]. On the other hand, these compounds are tremendously challenging to trace due to the too low sensitivity of the analytical methods and lack of standards [4,10,15].…”

Section: Introductionmentioning

confidence: 99%

“…Given that only about 25% of antibiotics are effectively used in aquaculture, the animal body poorly absorbs most antibiotics, and 30–90% of antibiotics are excreted via urine and feces into the environment. Consequently, antibiotics are frequently detected in surface water, groundwater, soils, and sediments [ 1 , 6 , 7 ].…”

Section: Introductionmentioning

confidence: 99%

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Heterogeneous Photocatalysis of Amoxicillin under Natural Conditions and High-Intensity Light: Fate, Transformation, and Mineralogical Impacts

Ellepola

Rubasinghege

2022

Environments

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The β-Lactam antibiotic amoxicillin is among the most widely used antibiotics in human and veterinary medicine. Consequently, amoxicillin is abundant in natural waters and can undergo diverse abiotic reactions to form degradation compounds under environmental conditions. Yet, little is known about these decay pathways and mineralogical impacts on environmental amoxicillin degradation. The current study focuses on understanding the mineralogical influences of amoxicillin degradation under ecological conditions. We studied the role of anatase and kaolinite on amoxicillin degradation under irradiated and non-irradiated conditions. Anatase increases amoxicillin degradation by 4.5-fold in the presence of light compared to just being exposed to sunlight. Interestingly, anatase also showed a higher degradation rate under dark than light controls. Conversely, kaolinite diminishes the amoxicillin degradation under irradiation. The formation of degradation compounds was mineralogy-controlled, while no mineralization was observed. Further, we irradiated amoxicillin with a high-intensity light to evaluate its removal from wastewater. The formation of varying amoxicillin degradation products with high-intensity light will limit its removal from wastewater. Our study emphasizes that the mineralogical impact on amoxicillin degradation is diverse, and the role of anatase is significant. Consequently, the increased addition of manufactured titanium nanoparticles to the environment can further enhance these effects.

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Bimetallic adsorbents for wastewater treatment: a review

et al. 2023

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Degradation of amoxicillin from water by ultrasound-zero-valent iron activated sodium persulfate

Cited by 40 publications

References 36 publications

Hydrothermal synthesis of magnetic nano-CoFe2O4 catalyst and its enhanced degradation of amoxicillin by activated permonosulfate

Hydrothermal synthesis of magnetic nano-CoFe2O4 catalyst and its enhanced degradation of amoxicillin by activated permonosulfate

Heterogeneous Photocatalysis of Amoxicillin under Natural Conditions and High-Intensity Light: Fate, Transformation, and Mineralogical Impacts

Bimetallic adsorbents for wastewater treatment: a review

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