Surface phonon cavities that are homogenous in both mechanical and dielectric properties are reported. The cavities are formed by the placement of a defect of a single domain within periodic domain inversion of single crystal piezoelectric lithium niobate that exhibits surface phononic bandgap through the phonon-polariton coupling. Surface cavity resonances are observed within the bandgap, which manifest in entrapment of phonon-polariton within the defect. In addition to demonstrating that the observed resonances are non-radiative and decoupled to bulk radiation, which is critical for high Q cavities, it is also shown the possibility to tune the surface cavity resonance spectra simply by varying the defect width. Such an ability to excite surface cavity resonance that is non-radiative with simultaneous localization of the electric field together with the advantage of a cavity that is physically formed from a completely monolithic and uniform material offers unique opportunities for widespread applications for example in actuation, detection, and phonon lasing that can be fully integrated with other physical systems such as quantum acoustics, photonics, and microfluidics.Phononic bandgap structures and phononic crystals are novel class of materials, which have emerged as promising candidates to control the suppression and redirection of phonon propagation in controlled manner in contrast to their behavior in unstructured bulk materials, given rise by their unique properties, namely phononic bandgaps [1-3] and negative refraction [4]. The ability for such control is crucial for current research in phonon-mediated photonic interactions [5][6][7][8][9], quantum physics [10-13], biosensing [14,15], and nano-scale thermal management [16,17]. A critical requirement in many of these applications is the ability to insulate a region of interest from random phonons in the environment. Reports have shown that if a defect is embedded within a phononic bandgap structure, a phonon cavity can be formed [18][19][20][21][22], enabling the trapping and concentration of phonons of a specific resonant frequency in a desired location, which has been observed via a picosecond ultrasonic technique [21], by Brillouin light scattering [19] or Raman spectra [18]. Dynamic tuning of these phonon cavity resonances can be directly achieved by controlling defect parameters, thus facilitating a number of applications, such as acoustic diodes [23], coherent phonon generation [20][21][22], thermal control [16,17], and concurrent phonon-photon modulation [24,25].The vast majority of the research [18][19][20][21][22], nevertheless, have been carried out to obtain phononic cavities for bulk waves; these structures typically comprising periodic composite media, often exclusively engineered from multi-layer single crystal semiconductor materials, achieved by molecular beam epitaxy. On the other hand, cavities for surface acoustic waves (SAWs) are highly desirable due to the enhanced concentration of acoustic energy at the surface that can facilitate di...