Abstract:Three binary dye mixtures prepared from the basic textile dyes Astrazon Blue FGRL (AB), Astrazon Red GTLN (AR), and Astrazon Golden Yellow GL-E (AY), were employed to demonstrate two different mixture characteristics. The first type of mixture (AB + AY) was the case where the optical absorbance spectra of the dye mixtures exhibited double peaks. Each peak occurred at the same wavelength as the single dye and the area under each light absorbance curve varied with the concentration of the dye in the solution. Th… Show more
“…2(e) and 2(f)). Since the surface band crosses the bulk band, it cannot be an eigenstate of the system but possibly a surface resonance state; this surface state is investigated further in smaller doping, x=0.001 samples [17]. We also note that in x = 0.01 samples a second bulk band is expected with a Fermi crossing near the surface band.…”
Much progress has been made recently in the study of the effects of electron-phonon (el-ph) coupling in doped insulators using angle resolved photoemission (ARPES), yielding evidence for the dominant role of el-ph interactions in underdoped cuprates. As these studies have been limited to doped Mott insulators, the important question arises how this compares with doped band insulators where similar el-ph couplings should be at work. The archetypical case is the perovskite SrTiO 3 (STO), well known for its giant dielectric constant of 10000 at low temperature, exceeding that of La 2 CuO 4 by a factor of 500. Based on this fact, it has been suggested that doped STO should be the archetypical bipolaron superconductor. Here we report an ARPES study from high-quality surfaces of lightly doped SrTiO 3 . Comparing to lightly doped Mott insulators, we find the signatures of only moderate electron-phonon coupling: a dispersion anomaly associated with the low frequency optical phonon with a λ ′ ∼ 0.3 and an overall bandwidth renormalization suggesting an overall λ ′ ∼ 0.7 coming from the higher frequency phonons. Further, we find no clear signatures of the large pseudogap or small polaron phenomena. These findings demonstrate that a large dielectric constant itself is not a good indicator of el-ph coupling and highlight the unusually strong effects of the el-ph coupling in doped Mott insulators.Strong energy-momentum dispersion in the lightly doped SrTiO 3 2
“…2(e) and 2(f)). Since the surface band crosses the bulk band, it cannot be an eigenstate of the system but possibly a surface resonance state; this surface state is investigated further in smaller doping, x=0.001 samples [17]. We also note that in x = 0.01 samples a second bulk band is expected with a Fermi crossing near the surface band.…”
Much progress has been made recently in the study of the effects of electron-phonon (el-ph) coupling in doped insulators using angle resolved photoemission (ARPES), yielding evidence for the dominant role of el-ph interactions in underdoped cuprates. As these studies have been limited to doped Mott insulators, the important question arises how this compares with doped band insulators where similar el-ph couplings should be at work. The archetypical case is the perovskite SrTiO 3 (STO), well known for its giant dielectric constant of 10000 at low temperature, exceeding that of La 2 CuO 4 by a factor of 500. Based on this fact, it has been suggested that doped STO should be the archetypical bipolaron superconductor. Here we report an ARPES study from high-quality surfaces of lightly doped SrTiO 3 . Comparing to lightly doped Mott insulators, we find the signatures of only moderate electron-phonon coupling: a dispersion anomaly associated with the low frequency optical phonon with a λ ′ ∼ 0.3 and an overall bandwidth renormalization suggesting an overall λ ′ ∼ 0.7 coming from the higher frequency phonons. Further, we find no clear signatures of the large pseudogap or small polaron phenomena. These findings demonstrate that a large dielectric constant itself is not a good indicator of el-ph coupling and highlight the unusually strong effects of the el-ph coupling in doped Mott insulators.Strong energy-momentum dispersion in the lightly doped SrTiO 3 2
“…These experiments provide opportunity for new investigations about the electronic order behind cuprates. In spite of different experiments showing similar features, the interpretation is not unique 5,6,7,8,9,10 . For instance, Xie et al 6 argue that, near the Fermi level, the quasiparticle band breaks at about ∼ −350meV and, at higher energies follows the dispersion predicted by band structure calculation.…”
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confidence: 91%
“…On the other hand, in Ref. [9], it was also obtained that high energy features lie at higher energies than the pre- vs ω in the full range of frequency. The self-energy is strongly asymmetric around ω = 0 reflecting differences between the addition and removal of a single electron in a correlated system.…”
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confidence: 93%
“…Recently, ARP ES measurements 5,6,7,8,9,10 reported results up to large energy ω ∼ −1eV , clearly showing the presence of high energy self-energy renormalizations contributing to the spectral functions. The extracted E − k dispersion from momentum distribution curves seems to show a nearly vertical "dive" 10 (also called "waterfall" 7 ) at about 350meV .…”
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confidence: 98%
“…In Σ, double dashed line, which contains collective charge fluctuations, can be seen as the excitations that interacting with fermions lead to the selfenergy effects and incoherent structures discussed in the text. excitations were identified but not compared with the new ARP ES experiments 5,6,7,8,9,10 which are more recent than Ref. [13].…”
We discuss first some basic experimental facts related to ARPES, tunnelling, optics ad neutron scattering measurements. They give evidence for the relevance of the electron-phonon interaction (EPI) in pairing mechanism of HTSC cuprates. A controllable and very efficient theory for strong correlations and their effects on EPI is discussed. The theory is based on the 1/N expansion method in the t-J model without using slave bosons (or fermions). The remarkable prediction is that strong correlations renormalize EPI and other charge-fluctuation properties (by including nonmagnetic impurity scattering) in such a way that the forward scattering peak (FSP) appears in the corresponding effective interactions. The existence of FSP in EPI is additionally supported by the weakly screened Madelung interaction in the ionic-metallic structure of layered cuprates. Pronounced FSP in EPI of HTSC cuprates reconciles many puzzling results, which could not be explained by the old theory with the momentum independent EPI. For instance, EPI with FSP gives that the couplings in the s-and d-wave pairing channel are of the same magnitude near and below the optimal hole doping. It is shown that FSP in the impurity scattering potential is responsible for robustness of d-wave pairing in cuprates with nonmagnetic impurities and other defects. The ARPES kink and the isotope effect in the nodal and anti-nodal points, as well as the collapse of the elastic nonmagnetic impurity scattering in the superconducting state, are explained by this theory in a consistent way. The proposed theory also explains why the nodal kink is not-shifted in the superconducting state while the anti-nodal kink is shifted by the maximal superconducting gap. It turns out that in systems with FSP in EPI besides the classical phase fluctuations there are also internal fluctuations of Cooper pairs. The latter effect is pronounced in systems with long-ranged pairing forces, thus giving rise to an additional contribution to the pseudogap behavior.PACS numbers:
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