Cyclic three-level-pulse-area theorem for enantioselective state transfer of chiral molecules
Yu Guo,
Xun Gong,
Songshan Ma
et al.
Abstract:We derive a pulse-area theorem for a cyclic three-level system, an archetypal model for exploring enantioselective state transfer (ESST) in chiral molecules driven by three linearly polarized microwave pulses.By dividing the closed-loop excitation into two separate stages, we obtain both amplitude and phase conditions of three control fields to generate high fidelity of ESST. As a proof of principle, we apply this pulse-area theorem to the cyclohexylmethanol molecules (C 7 H 14 O), for which three rotational s… Show more
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