Abstract:Graphdiyne (GDY) is an artificial carbon allotrope that is conceptually similar to graphene but composed of sp- and sp2-hybridized carbon atoms. Monolayer GDY (ML-GDY) is predicted to be an ideal two-dimensional (2D) semiconductor material with a wide range of applications. However, its preparation has not been achieved experimentally due to difficulties with synthesis. Here, we report that in-situ polymerization of hexaethynylbenzene within the sub-nanometer interlayer space of MXene can effectively prevent o… Show more
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