Abstract:The molecular spin-crossover, SCO, phenomenon, involving thermo-, photo-and piezo-chromic properties of a class of transition-metal complexes (3d 4 -3d 7 ), is one of growing importance in the area of functional materials, especially for application as molecular switches and in the field of information storage. These complexes are known to display a molecular bistability of high-spin (HS) and low-spin (LS) electronic configurations, which are distinguished by different occupation of antibonding e g and bonding… Show more
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