The eastern North American margin (ENAM; Figure 1a) represents an archetypical passive margin, which experienced the assembly and breakup of the supercontinent Pangea over the last 500 Ma (Thomas, 2006). During the assembly of Pangea between ∼495 Ma and ∼270 Ma, a sequence of tectonic terranes progressively accreted onto the North American craton (namely Laurentia) (Hatcher, 2010;Thomas, 2006). Extensive rifting along the ENAM started at ∼230 Ma (Withjack et al., 2012), and was accompanied by short-lived igneous activities. Enormous postrifting magmatism occurred over a period of less than 1 million years at ∼200 Ma and formed one of the Earth's largest igneous provinces, the Central Atlantic Magmatic Province (Marzoli et al., 1999(Marzoli et al., , 2018. Rifting led to the breakup of Pangea at ∼185 Ma, and the modern passive margin was ultimately established (Withjack et al., 2012).The southern segment of the ENAM is characterized by a variety of tectonic features associated with both syn-and postrifting tectonic events. For example, a positive magnetic anomaly (namely the East Coast Magnetic Anomaly) aligns approximately in the SW-NE direction (Figures 1 and S1a). The East Coast Magnetic Anomaly likely represents volcanism that was associated with the initial rifting at ∼230 Ma, and thus marks the boundary between the oceanic and continental lithosphere (Austin et al., 1990;Klitgord