Abstract:We investigate the electrical conductance of long, high-mobility quantum wires formed by the split-gate technique, which allows for adjustment of the wire width and the number of one-dimensional electron subbands, n. In wires with 3 Show more
“…High-pressure XAS experiments were performed for osmium by investigating the X-ray absorption near edge structure (XANES) at beamline 20-BM-B of the APS. A panoramic DAC 12 with 400 μm diamonds was used to collect spectra at both the L 2 and L 3 absorption edges for the Na 2 OsO 4 powders. In order to avoid contamination of the XANES spectra by Bragg peaks from the diamond anvils, XANES measurements were performed in transmission geometry where the X-ray beam goes through a beryllium gasket.…”
Section: Experimental and Computational Methodsmentioning
confidence: 99%
“…1e). As mentioned above, the interacting fermions in one spatial dimension do not obey FL theory; however, the possibility of the deconfinement transition induced by interchain hopping [11] or a transition to a weakly disordered Fermi liquid [12] for more higher pressures cannot be neglected as alters with pressure strongly towards FL state.…”
Na 2 OsO 4 is an unusual quantum material that, in contrast to the common 5d 2 oxides with spins = 1, owns a magnetically silent ground state with spin = 0 and a band gap at Fermi level attributed to a distortion in the OsO 6 octahedral sites. In this semiconductor, our low-temperature electrical transport measurements indicate an anomaly at 6.3 K with a power-law behavior inclining through the semiconductor-to-metal transition observed at 23 GPa. Even more peculiarly, we discover that before this transition, the material becomes more insulating instead of merely turning into a metal according to the conventional wisdom. To investigate the underlying mechanisms, we applied experimental and theoretical methods to examine the electronic and crystal structures comprehensively, and conclude that the enhanced insulating state at high pressure originates from the enlarged distortion of the OsO 6 . It is such a distortion that widens the band gap and decreases the electron occupancy in Os's t 2g orbital through an interplay of the lattice, charge, and orbital in the material, which is responsible for the changes observed in our experiments.
“…High-pressure XAS experiments were performed for osmium by investigating the X-ray absorption near edge structure (XANES) at beamline 20-BM-B of the APS. A panoramic DAC 12 with 400 μm diamonds was used to collect spectra at both the L 2 and L 3 absorption edges for the Na 2 OsO 4 powders. In order to avoid contamination of the XANES spectra by Bragg peaks from the diamond anvils, XANES measurements were performed in transmission geometry where the X-ray beam goes through a beryllium gasket.…”
Section: Experimental and Computational Methodsmentioning
confidence: 99%
“…1e). As mentioned above, the interacting fermions in one spatial dimension do not obey FL theory; however, the possibility of the deconfinement transition induced by interchain hopping [11] or a transition to a weakly disordered Fermi liquid [12] for more higher pressures cannot be neglected as alters with pressure strongly towards FL state.…”
Na 2 OsO 4 is an unusual quantum material that, in contrast to the common 5d 2 oxides with spins = 1, owns a magnetically silent ground state with spin = 0 and a band gap at Fermi level attributed to a distortion in the OsO 6 octahedral sites. In this semiconductor, our low-temperature electrical transport measurements indicate an anomaly at 6.3 K with a power-law behavior inclining through the semiconductor-to-metal transition observed at 23 GPa. Even more peculiarly, we discover that before this transition, the material becomes more insulating instead of merely turning into a metal according to the conventional wisdom. To investigate the underlying mechanisms, we applied experimental and theoretical methods to examine the electronic and crystal structures comprehensively, and conclude that the enhanced insulating state at high pressure originates from the enlarged distortion of the OsO 6 . It is such a distortion that widens the band gap and decreases the electron occupancy in Os's t 2g orbital through an interplay of the lattice, charge, and orbital in the material, which is responsible for the changes observed in our experiments.
“…The numerical self-consistent approach can be used to solve the coupled equations, which accurately predicts the electrostatic potential profile (band bending) arising from various sources (such as ionized dopants, surface charges, and external gates) [5][6][7]. Such self-consistent solutions offer information on spatial-dependent observables, such as wavefunctions and electron density [8], which can be used to estimate the size of a quantum well [9,10].…”
Achieving self-consistent convergence with the conventional effective-mass approach at ultra-low temperatures (below 4.2 K) is a challenging task, which mostly lies in the discontinuities in material properties (e.g., effective-mass, electron affinity, dielectric constant). In this article, we develop a novel self-consistent approach based on cell-centered Finite-Volume discretization of the Sturm-Liouville form of the effective-mass Schrödinger equation and generalized Poisson's equation (FV-SP). We apply this approach to simulate the one-dimensional electron gas (1DEG) formed at the Si-SiO2 interface via a top gate. We find excellent self-consistent convergence from high to extremely low (as low as 50 mK) temperatures. We further examine the solidity of FV-SP method by changing external variables such as the electrochemical potential and the accumulative top gate voltage. Our approach allows for counting electron-electron interactions. Our results demonstrate that FV-SP approach is a powerful tool to solve effective-mass Hamiltonians.
“…Furthermore, quantitative knowledge from the coupled equations on the quantized energy ladder, penetration of wavefunctions (envelope functions) in the potential barrier (oxide), and occupation factors can provide essential information on the interpretation of experimental data and optimization of nanoscale semiconductor devices [9][10][11][12][13]. In addition, the coupled equations offer information on spatial-dependent observables, such as wavefunctions and electron density [14], which can be used to estimate the size of a quantum well [15,16].…”
The conventional (numerical) Self-Consistent effective-mass approaches suffer from convergence failure at ultra-low temperatures (below 4.2 K). Discontinuities in material properties (e.g., effectivemass, electron affinity, dielectric constant) can be regarded as the source of such a shortcoming. This numerical convergence sensitivity limits the application of Self-Consistent effective-mass approach to study quantum electronic devices which often operate at ultra-low temperatures. In this article, we develop a novel Self-Consistent approach based on Cell-Center Finite-Volume (FV-SC) discretization of the effective-mass Sturm-Liouville Hamiltonian and generalized Poisson's equation. We apply this approach to simulate the one-dimensional electron gas (1DEG) formed at the Si-SiO2 interface via a top gate. We find excellent Self-Consistent convergence from high to extreme low (as low as 50 mK) temperatures. We further examine the solidity of FV-SC method by changing external variables such as the electrochemical potential and the accumulative top gate voltage. Finally, our approach allows for counting electron-electron interactions and we find that the electron-electron interactions can affect the subband properties of 1DEG significantly. Our results demonstrate that our FV-SC approach is a powerful tool to solve effective-mass Hamiltonian.
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