Critical Investigation of Metal–Organic-Frameworks to Improve the Silicon Anode of Lithium-Ion Batteries
James W. Sturman,
Mohamed S. E. Houache,
Walace Doti do Pim
et al.
Abstract:The poor capacity retention of the silicon (Si) anode has hindered its widespread use in lithium-ion batteries. Metal− organic-frameworks (MOF) may offer the structural and functional tunability needed to alleviate some of the longstanding problems associated with silicon pulverization. Herein, MOF-74 (Co-based) and were implemented in different design configurations for high-Si loading electrodes. Multilayer sandwich configurations provided a modest improvement in capacity retention. However, greatest improv… Show more
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