The Gusandong Tuff (Kusandong Tuff), known as a very significant key bed in the Cretaceous Gyeongsang Basin, is divided into (1) Northern Gusandong Tuff (NKT), (2) Southern Gusandong Tuff (SKT), and (3) Sinsudo Tuff, which were derived from different vents. In order to suggest their more accurate eruption times and to contribute to establishing stratigraphy of the basin, SHRIMP U-Pb zircon ages were determined from the three tuffs. As a result, the virtually same ages of 103.0±1.2 Ma and 104.1±1.3 Ma were obtained from NKT and SKT, respectively, which mean that they simultaneously erupted during 103~104 Ma. The zircon ages obtained from the Sinsudo Tuff are however divided into two groups i.e. 103.4±2.1 and 95.79±0.98 Ma. Based on distinctive morphology and cathodoluminescence image of the younger zircons, the younger age, 95.79±0.98 Ma, is much more reasonable as the eruption time of the Sinsudo Tuff.