Graphene, because of the prominent mechanical strength, [17] high electric and thermal conductivity, [18] and high carrier mobility, [19][20][21] has received ever-growing interest in creating pressure sensors, [22,23] together with other candidates like carbon nanotubes (CNTs), [24,25] metallic nanowires, [26] and polypyrrole. [27] Wavy graphene structure can form periodic wrinkles and is considered as one type of skin-inspired crumpled structures, which can be fabricated by the pattern-assisted method [28] and the pre-strain method. [29] Wavy graphene materials have been widely applied in diverse applications, for example, capacitors [30] and strain sensors. [31] However, the wavy graphene structure, especially the one with gradient feature, has not attracted enough attention for developing novel pressure sensors.In this work, we prepared wavelength-gradient graphene films to exhibit the gradient feature and other conventional properties of pressure sensors. Due to the gradient structure, the electrical conductivity in the sensors increased when applying equal pressures on different areas where the average wavelength of the wrinkles increased. And the pressure sensor also exhibited a high sensitivity toward external pressure in a wide range (0-5000 Pa), a low limit of detection of 24.5 Pa, and a slow response time of ≈1 s. Accordingly, we further anticipate the novel pressure sensor to find practical applications in detecting the position of equal pressures and in amplifying the difference of electric signal of two similar pressures, due to the pressure-sensitive performance of the unique gradient structure. Figure 5. a) The detection limit of the pressure sensor and its response time. b) Current change of the pressure sensor at different pressure of 49, 122.5, 367.5, and 980 Pa. c) Current change of the pressure sensor under a pressure of 2 kPa at a frequency of 0.025 Hz for 500 cycles, and current change of the pressure sensor restarting after a 30 min pause. www.advancedsciencenews.com