The directional angular correlations of the 208.36-112.97 kev gamma-gamma cascade in Hf 177 and the 89. 36-343.40 and 282.57-113.81 kev cascades in Lu 175 have been measured with a coincidence scintillation spectrometer using Nal detectors. The observed correlation functions obtained with dilute aqueous solution sources are IF(0) = 1-(O.1614±O.OO15)P 2 (cos0), W(d) = l + (0.001 ±O.OO4)P 2 (cos0), and W(d) = l + (O.221±O.OO4)J? 2 (cos0), respectively.These results, taken together with conversion coefficient measurements, indicate that 5 2 for the 282.57-kev gamma ray in Lu 175 is 0.05. The sign of 8, defined below, is positive. The mixing ratio of the 208.36-kev gamma ray in Hf 177 is M2/El=0.001; in this case the sign of 8 is negative. The sign of 8 for the 113.81-kev gamma ray in Lu 175 is positive, and the sign of 8 for the 112.97-kev gamma ray in Hf 177 is negative.