Abstract:Pure UO2 pellets and, for the first time, AGR SIMFUEL pellets simulating 25 (pellet interior) and 43 GWd/tU burn-up (rim structure) have been fabricated. Using combined electrochemical and Raman spectroscopic studies, we have investigated the effect of the AGR SIMFUEL dopants on the structure of the UO2 crystal matrix and studied the effect of H2O2 on the SIMFUEL surface as a simulant for the effect of α radiolysis of water within intruding groundwater in the near field. Preliminary results of electrochemical … Show more
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