Interfacial solar steam generation (ISSG) has recently
received
much attention as a low-carbon-footprint and high-energy-efficient
strategy for seawater desalination and wastewater treatment. However,
achieving the goals of a high evaporation rate, ecofriendliness, and
high tolerance to salt ions in brine remains a bottleneck. Herein,
a novel hydrogel-based evaporator for effective solar desalination
was synthesized on the basis of sodium alginate (SA) and carboxymethyl
chitosan (CMCS) incorporating a carbon nanotube (CNT)-wrapped melamine
sponge (MS) through a simple dipping–drying–cross-linking
process. The hydrogel-based evaporator reaches a high evaporation
rate of 2.18 kg m–2 h–1 in 3.5
wt % brine under 1 sun irradiation. Furthermore, it demonstrated excellent
salt ion rejection in high-concentration salt water. Simultaneously,
it exhibits excellent purification functionality toward heavy metals
and organic dyes. This study provides a simple and efficient strategy
for seawater desalination and wastewater treatment.