2014
DOI: 10.1103/physreve.89.062411
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Cooperative sequential-adsorption model in two dimensions with experimental applications for ionic self-assembly of nanoparticles

Abstract: Self-assembly of nanoparticles is an important tool in nanotechnology, with numerous applications, including thin films, electronics, and drug delivery. We study the deposition of ionic nanoparticles on a glass substrate both experimentally and theoretically. Our theoretical model consists of a stochastic cooperative adsorption and evaporation process on a two-dimensional lattice. By exploring the relationship between the initial concentration of nanoparticles in the colloidal solution and the density of parti… Show more

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Cited by 10 publications
(5 citation statements)
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“…We believe that our approach may be useful for future experimental work because it suggests a procedure to identify the characteristic time τ and shows how the adsorbate features at times of this order are related to polydispersity. Our results may also be useful in future RSA studies, for instance to models including particle interactions, particle mobility, and other particle shapes and substrate structures [54,55]. The detailed study of features at times of order τ may also be interesting in off-lattice (continuum) RSA, for instance considering the variety of particle shapes studied in recent works for modeling compact and branched structures [56,57].…”
Section: Discussionmentioning
confidence: 73%
“…We believe that our approach may be useful for future experimental work because it suggests a procedure to identify the characteristic time τ and shows how the adsorbate features at times of this order are related to polydispersity. Our results may also be useful in future RSA studies, for instance to models including particle interactions, particle mobility, and other particle shapes and substrate structures [54,55]. The detailed study of features at times of order τ may also be interesting in off-lattice (continuum) RSA, for instance considering the variety of particle shapes studied in recent works for modeling compact and branched structures [56,57].…”
Section: Discussionmentioning
confidence: 73%
“…The deposition rate depends on the number of occupied neighbours. A complete derivation of this equation can be found in Cook et al [13].…”
Section: Rate Equation For the Particle Densitymentioning
confidence: 99%
“…After relating the model parameters to physical ones, we are able to use our model to create films with specific particle densities. For example, the concentration of the colloidal suspension was linked to the level of particle interaction and the final particle density in a recent paper [13].…”
Section: Two-dimensional Lattice and Ionic Self-assembly Of Nanoparti...mentioning
confidence: 99%
“…Noncontact manipulation plays a significant role in a large number of modern scientific and technological fields, such as biophysics [1], life science [2,3], and nanotechnology [4]. Since Ashkin's pioneering work on optical tweezers was performed in the early 1970s [5], optical tweezers have become a favorite way to manipulate particles.…”
Section: Introductionmentioning
confidence: 99%