Conversion of nitrogenous small molecules into value-added chemicals by building N–C bonds

Zhang, Yuanyuan; Yu, Qian; Wang, Xin; Guo, Wei

doi:10.1016/j.cej.2023.145899

Chemical Engineering Journal

2023

DOI: 10.1016/j.cej.2023.145899

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Conversion of nitrogenous small molecules into value-added chemicals by building N–C bonds

Yuanyuan Zhang,

Qian Yu,

Xin Wang

et al.

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2024

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Cited by 2 publications

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Electrocatalytic synthesis of C–N coupling compounds from CO₂ and nitrogenous species

Zhang,

Li,

et al. 2024

SusMat

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The electrocatalytic synthesis of C–N coupling compounds from CO2 and nitrogenous species not only offers an effective avenue to achieve carbon neutrality and reduce environmental pollution, but also establishes a route to synthesize valuable chemicals, such as urea, amide, and amine. This innovative approach expands the application range and product categories beyond simple carbonaceous species in electrocatalytic CO2 reduction, which is becoming a rapidly advancing field. This review summarizes the research progress in electrocatalytic urea synthesis, using N2, NO2−, and NO3− as nitrogenous species, and explores emerging trends in the electrosynthesis of amide and amine from CO2 and nitrogen species. Additionally, the future opportunities in this field are highlighted, including electrosynthesis of amino acids and other compounds containing C–N bonds, anodic C–N coupling reactions beyond water oxidation, and the catalytic mechanism of corresponding reactions. This critical review also captures the insights aimed at accelerating the development of electrochemical C–N coupling reactions, confirming the superiority of this electrochemical method over the traditional techniques.

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Electrocatalytic synthesis of C–N coupling compounds from CO₂ and nitrogenous species

Zhang,

Li,

et al. 2024

SusMat

View full text Add to dashboard Cite

show abstract

Prediction of molecular-specific mutagenic alerts and related mechanisms of chemicals by a convolutional neural network (CNN) model based on SMILES split

Chen,

Huang,

Zou

et al. 2024

Science of The Total Environment

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Conversion of nitrogenous small molecules into value-added chemicals by building N–C bonds

Cited by 2 publications

References 103 publications

Electrocatalytic synthesis of C–N coupling compounds from CO₂ and nitrogenous species

Electrocatalytic synthesis of C–N coupling compounds from CO₂ and nitrogenous species

Prediction of molecular-specific mutagenic alerts and related mechanisms of chemicals by a convolutional neural network (CNN) model based on SMILES split

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Conversion of nitrogenous small molecules into value-added chemicals by building N–C bonds

Cited by 2 publications

References 103 publications

Electrocatalytic synthesis of C–N coupling compounds from CO2 and nitrogenous species

Electrocatalytic synthesis of C–N coupling compounds from CO2 and nitrogenous species

Prediction of molecular-specific mutagenic alerts and related mechanisms of chemicals by a convolutional neural network (CNN) model based on SMILES split

Contact Info

Product

Resources

About

Electrocatalytic synthesis of C–N coupling compounds from CO₂ and nitrogenous species

Electrocatalytic synthesis of C–N coupling compounds from CO₂ and nitrogenous species