Conversion of Nitrate to Ammonia by Amidinothiourea-Coordinated Metal Molecular Electrocatalysts with d−π Conjugation
Xue-Bo Liu,
Rui Zhao,
Min-Min Xu
et al.
Abstract:The electrochemical reduction of nitrate to ammonia (NO 3 RR) provides a desired alternative of the traditional Haber−Bosch route for ammonia production, igniting a research boom in the development of electrocatalysts with high activity. Among them, molecular electrocatalysts hold considerable promise for the NO 3 RR, suppressing the competing hydrogen evolution reaction. However, the complicated synthesis procedure, usage of environmentally unfriendly organic solvents, and poor stability of Cu-based molecular… Show more
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