Abstract:It remains challenging to control the single-, two-, and three-photon excited fluorescence of metal nanoclusters. In this work, the control over the nonlinear optics of metal nanoclusters as single-, two-, and three-photon excited fluorescence has been accomplished via exploiting the solvent effect. An emissive nanocluster, Au 9 Ag 6 (SPh t OMe) 4 (DPPOE) 3 Cl 3 , was synthesized and structurally determined. The solvent effect can not only control the fluorescence of this nanocluster, but more significantly, i… Show more
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