In the first part of this paper we shall classify proper triharmonic isoparametric surfaces in 3-dimensional homogeneous spaces (Bianchi-Cartan-Vranceanu spaces, shortly BCV-spaces). We shall also prove that triharmonic Hopf cylinders are necessarily CMC.In the last section we shall determine a complete classification of CMC r-harmonic Hopf cylinders in BCV-spaces, r ≥ 3. This result ensures the existence, for suitable values of r, of an ample family of new examples of r-harmonic surfaces in BCV-spaces.