2017
DOI: 10.1016/j.compositesa.2017.06.003
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Conductive thermoplastic polyurethane composites with tunable piezoresistivity by modulating the filler dimensionality for flexible strain sensors

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Cited by 164 publications
(116 citation statements)
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References 49 publications
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“…There are three main reported strategies: (1) inltrating elastomers with conductive ller networks, 9,10,28,29 (2) synthesizing metal llers within elastomers 3,28,[30][31][32] and (3) implanting conductive llers into elastomers. 12,21,22,26,27,[33][34][35][36][37][38][39][40][41][42][43][44][45] The rst strategy generally requires particular fabrication techniques, such as surface treatment, to assist the combination of elastomers with conductive llers. Besides, conductive ller networks built on the surface or in the subsurface of the elastomers may be damaged under long-term high-level strain service duration due to the weak bonding between ller networks and elastomers.…”
Section: Introductionmentioning
confidence: 99%
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“…There are three main reported strategies: (1) inltrating elastomers with conductive ller networks, 9,10,28,29 (2) synthesizing metal llers within elastomers 3,28,[30][31][32] and (3) implanting conductive llers into elastomers. 12,21,22,26,27,[33][34][35][36][37][38][39][40][41][42][43][44][45] The rst strategy generally requires particular fabrication techniques, such as surface treatment, to assist the combination of elastomers with conductive llers. Besides, conductive ller networks built on the surface or in the subsurface of the elastomers may be damaged under long-term high-level strain service duration due to the weak bonding between ller networks and elastomers.…”
Section: Introductionmentioning
confidence: 99%
“…In our previous work, it was found that the formation of segregated CNS networks at the interface of thermoplastic polyurethane (TPU), which is a widely used elastomer for exible sensors, 17,25,39,42,44,68,69 is able to signicantly reduce F C of the TPU/CNS composites in comparison with melt mixing. 70 Besides, the elastomer particle size plays an important role in controlling the ller network morphology in the segregated network structure, affecting the composite's electrical and mechanical properties.…”
Section: Introductionmentioning
confidence: 99%
“…In general, CNTs tend to be entangled in polymer matrix . This entanglement phenomenon seriously affects the integrity of composites.…”
Section: Resultsmentioning
confidence: 99%
“…Stretchability can be very diverse, depending on elasticity of the substrates/matrix, the type of nanomaterials, structure of the sensors/conductors, and fabrication process. For nanocomposite‐based sensors containing nanomaterials of different dimensions (0D, 1D, or 2D), those based on 0D nanoparticles generally show higher sensitivity but lower stretchability . There are several mechanisms contributing to the piezoresistivity of nanocomposite‐based sensors, including disconnection mechanisms (e.g., loss of contact), tunneling resistance change due to interparticle distance changes, and intrinsic piezoresistivity of nanomaterials.…”
Section: Characteristics Of Stretchable Strain Sensors/conductorsmentioning
confidence: 99%