Abstract:Resonant molecular optical second harmonic generation (SHG) has been obtained from [2,3,7,8,12, 13, 17, vanadyl, (OEP)V=O, adsorbed on the hypotenuse face of a glass prism. Rotational intensity patterns are showed by plotting the second harmonic intensity as a function of the incident polarization angle of the fundamental wave, at a fixed angle of incidence. Evaluation of these patterns by Fourier analysis allowed the determination of the second order susceptibilities components of the adsorbed layers. Assumin… Show more
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