“…Indeed many approaches to produce neutral free-radical beams have been developed also in the fields of experimental chemistry [1], heating of plasmas for controlled thermonuclear fusion, and experimental simulation of low-earth orbit phenomena [2J, but efficient production of the steady-flux refined beam of neutral free radicals ( RBNR ) has not been realized yet. In order to overcome the difficulty we have proposed several experimental production approaches, two of which are photo-deionization of negative ion beams ( PDINIB ) [3,4] and photo-dissociation of energetic compound beams ( PDECB ) [5,6. We have been developing a trial surface processing apparatus utilizing a steady-flux RBNR produced according to the following PDINIB procedure. Firstly, a steady-flux negative ion beam ( NIB ) of the desired chemical species generated by the high 0 100 current density negative ion source is purified at the mass separator LB Then, immediately after it is decelerated to the desired kinetic energy and made convergent by the triple-electrode decelerator at Fig.!.…”