A graph is called set-sequential if its vertices can be labeled with distinct nonzero vectors in F n 2 such that when each edge is labeled with the sum (mod 2) of its vertices, every nonzero vector in F n 2 is the label for either a single vertex or a single edge. We resolve certain cases of a conjecture of Balister, Győri, and Schelp in order to show many new classes of trees to be set-sequential. We show that all caterpillars T of diameter k such that k ≤ 18 or |V (T )| ≥ 2 k−1 are set-sequential, where T has only odd-degree vertices and |T | = 2 n−1 for some positive integer n. We also present a new method of recursively constructing set-sequential trees.