Abstract:Grain boundaries (GBs) are vital to crystal materials and their applications. Although the GBs in bulk and two-dimensional materials have been extensively studied, the polyline GBs prevalently forming in transition metal dichalcogenide monolayers by a sequence of folded segments remain a mystery. We visualize the large-area distribution of the polyline GBs in MoSe2 monolayers by means of a strain mapping method and unravel their structural origin using ab initio calculations combined with high-resolution atomi… Show more
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