Coating Parameters That Influence the Defect Ratio of TRISO Coated Fuel Particles

Hancke, Jacobus J.; Barry, John C.; Rooyen, G. T. Van; Villiers, J. P. R. de

doi:10.13182/nt12-a14630

Cited by 3 publications

(2 citation statements)

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“…Reviews of the functions of the different layers of the TRISO particle are given by Wichner et al [32] and van der Berg et al [33]. CVD (chemical vapour deposition) processes are used to manufacture the layers [32,34]. Using high purity precursor chemicals ensure that the very low levels of impurities needed in a nuclear fission reactor is obtained.…”

Section: Coated Nuclear Fuel Particles (Triso Particles)mentioning

confidence: 99%

“…Symmetrical spherical particles are needed because asymmetrical ones have a higher probability of failure [36 -38]. The chemicals and deposition parameters are given in reference [32,34,35]. Examples of the characterization of the microstructure of the layers to determine whether the layers have the required properties are given in references [33, 34, 39 -45].…”

Section: Coated Nuclear Fuel Particles (Triso Particles)mentioning

confidence: 99%

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Diffusion of fission products and radiation damage in SiC

Malherbe

2013

J. Phys. D: Appl. Phys.

107

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A major problem with most of the present nuclear reactors is their safety in terms of the release of radioactivity into the environment during accidents. In some of the future nuclear reactor designs, i.e. Generation IV reactors, the fuel is in the form of coated spherical particles, i.e. TRISO (acronym for Triple Coated Isotropic) particles. The main function of these coating layers is to act as diffusion barriers for radioactive fission products, thereby keeping these fission products within the fuel particles, even under accident conditions. The most important coating layer is composed of polycrystalline 3C-SiC. This paper reviews the diffusion of the important fission products (silver, caesium, iodine and strontium) in SiC. Because radiation damage can induce and enhance diffusion, the paper also briefly reviews damage created by energetic neutrons and ions at elevated temperatures, i.e. the temperatures at which the modern reactors will operate, and the annealing of the damage. The interaction between SiC and some fission products (such as Pd and I) is also briefly discussed. As shown, one of the key advantages of SiC is its radiation hardness at elevated temperatures, i.e. SiC is not amorphized by neutron or bombardment at substrate temperatures above 350°C. Based on the diffusion coefficients of the fission products considered, the review shows that at the normal operating temperatures of these new reactors (i.e. less than 950°C) the SiC coating layer is a good diffusion barrier for these fission products. However, at higher temperatures the design of the coated particles needs to be adapted, possibly by adding a thin layer of ZrC.

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