2008
DOI: 10.5194/acpd-8-12721-2008
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Cloud processing, cloud evaporation and Angström exponent

Abstract: Abstract. With a cloud parcel model we investigated how cloud processing and cloud evaporation modify the size distribution and the Angström exponent of an aerosol population. Cloud processing causes a decrease in particle concentrations, relatively most efficiently in the coarse mode, and reduces the relative dispersion of the aerosol distribution. As a result the Angström exponent of the aerosol increases. The Angström exponent is subject to other influences. It is very sensitive for relative humidity, espec… Show more

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Cited by 5 publications
(7 citation statements)
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“…The exchange between cloudy air and environmental air, including the activated and unactivated aerosol particles, must therefore be represented realistically in atmospheric models aimed to study indirect aerosol effects. Further, due to entrainment of aerosol into clouds more particles will be subject to cloud processing (e.g., Roelofs and Kamphuis, 2009) which is relevant for the aerosol direct effect.…”
Section: Discussionmentioning
confidence: 99%
See 1 more Smart Citation
“…The exchange between cloudy air and environmental air, including the activated and unactivated aerosol particles, must therefore be represented realistically in atmospheric models aimed to study indirect aerosol effects. Further, due to entrainment of aerosol into clouds more particles will be subject to cloud processing (e.g., Roelofs and Kamphuis, 2009) which is relevant for the aerosol direct effect.…”
Section: Discussionmentioning
confidence: 99%
“…Since the initial CDNC is determined directly at cloud base, understanding how meteorological characteristics and aerosol properties influence aerosol activation at the cloud base has received a lot of attention (e.g., Kulmala et al, 1993). In the second place, the distribution of the liquid water with droplet size further influences both scattering and precipitation formation processes (e.g., Roelofs and Jongen, 2004;Roelofs and Kamphuis, 2009). A model study of cloud microphysics therefore requires a realistic representation of both CDNC and the drop size distribution.…”
Section: Introductionmentioning
confidence: 99%
“…Regions of enhanced humidity have the greatest horizontal extent near cloud top when an overlying stable layer exists [Perry and Hobbs, 1996;Lu et al, 2003], which in the tropics occurs around an altitude of 2 km [Rauber et al, 2007]. Also at cloud top, detrained cloud drops evaporate and leave behind larger, but fewer, aerosols compared to the entrained air due to droplet collision-coalescence within the cloud [Roelofs and Kamphuis, 2009]. Collision-coalescence occurs more often in thicker clouds, so its impact on aerosol size and hence, backscatter, is greatest at the tops of thicker clouds.…”
Section: Resultsmentioning
confidence: 99%
“…Hygroscopic growth increases both the median radius R and width s, leaving number concentration N unchanged [Gerber, 1985]. Droplet collision-coalescence decreases N and increases R, though precipitation scavenging efficiently removes the largest cloud droplets, thereby decreasing s [Peter et al, 2006;Roelofs and Kamphuis, 2009] and limiting the in-crease in R. Other scavenging processes (nucleation, diffusion, and impaction scavenging) decrease N and increase s [Flossmann et al, 1985]. We perform backscatter calculations to understand what changes in a typical maritime aerosol size distribution would produce our observations in Table 1.…”
Section: Resultsmentioning
confidence: 99%
“…Such a size is typical for water droplets in clouds 27,29 . Therefore, we attribute these values to water aerosols (fog, orographic clouds) present close to mountain's surface, also typical for the season in that area, as indicated by the meteorological data.…”
Section: Time-averaged Aerosol-backscattering-related ǻNgström Exponentmentioning
confidence: 99%