Chirality-Induced Electrical Generation of Magnetism in Nonmagnetic Elemental Tellurium

Abstract

Chiral matter has a structure that lacks inversion, mirror, and rotoreflection symmetry; thus, a given chiral material has either a right-or left-handed structure. In chiral matter, electricity and magnetism can be coupled in an exotic manner beyond the classical electromagnetism (e.g., magneto chiral effect in chiral magnets). In this paper, we give a firm experimental proof of the linear electric-current-induced magnetization effect in bulk nonmagnetic chiral matter elemental trigonal tellurium. We measured a 125 Te nuclear magnetic resonance (NMR) spectral shift under a pulsed electric current for trigonal tellurium single crystals. We provide general symmetry considerations to discuss the electrically (electric-field-and electric-current-) induced magnetization and clarify that the NMR shift observed in trigonal tellurium is caused by the linear current-induced magnetization effect, not by a higher-order magnetoelectric effect. We also show that the current-induced NMR shift is reversed by a chirality reversal of the tellurium crystal structure. This result is the first direct evidence of crystal-chirality-induced spin polarization, which is an inorganic-bulk-crystal analogue of the chirality-induced spin selectivity in chiral organic molecules. The present findings also show that nonmagnetic chiral crystals may be applied to spintronics and coil-free devices to generate magnetization beyond the classical electromagnetism.

Theory of Chiral Transport in Carbon Nanotubes

“…Thus the chiral response within the linear response is described as M = CJ with constant C, and J being the current along the tube axis. This response is called kinetic magnetoelectric effect and orbital Edelstein effect, 20,21,[24][25][26][27][28][29][30][31][32] and has been studied in the threedimensional bulk metals 20,21 and in topological insulators. 22 This effect is an orbital analog of the spin Edelstein effect.…”

Kinetic magnetoelectric effect in topological insulators

“…In recent years, new responses leading to orbital magnetization have been proposed in systems without inversion symmetry [1][2][3][4][5][6][7][8][9][10][11][12][13][14][15][16] . One of the focuses is conversion of electron current and magnetization on crystal structure with low symmetry.…”