Magnetically
actuated soft millirobots (magneto-robot) capable
of accomplishing on-demand tasks in a remote-control manner using
noninvasive magnetic fields are of great interest in biomedical settings.
However, the solid magneto-robots are usually restricted by the limited
deformability due to the predesigned shape, while the liquid magneto-robots
are capable of in situ shape reconfiguration but limited by the low
stiffness and geometric instability due to the fluidity. Herein, we
propose a magneto-active solid–liquid state transformable millirobot
(named MRF-Robot) made from a magnetorheological fluid (MRF). The
MRF-Robot can transform freely and rapidly between the Newtonian fluid
in the liquid state upon a weak magnetic field (∼0 mT) and
the Bingham plasticity in the solid state upon a strong magnetic field
(∼100 mT). The MRF-Robot in the liquid state can realize diverse
behaviors of large deformation, smooth navigation, in situ splitting,
merging, and gradient pulling actuated by a weak magnetic field with
a high gradient. The MRF-Robot in the solid state is distinguished
for the controllable locomotion with reconfigured shapes and versatile
object manipulations (including pull, push, and rotate the objects)
driven by a strong magnetic field with a high gradient. Moreover,
the MRF-Robot could continuously maneuver to accomplish diverse tasks
in the comprehensive scenes and achieve liquid-drug delivery, thrombus
clearance, and fluid-flow blockage in the phantom vascular model under
magnetic actuation.