“…CO(v) significantly grows after oxygen is added (see e.g. [25,52,53] and references there). As that is not the case, one may deduce that (R13) is not a major channel of CN(B) production.…”
Section: Concentrations Of Cn Molecule In the Excited B 2 R Statementioning
The emission by electronically excited CN molecules is a prominent feature in the spectrum of active nitrogen containing traces of carbonaceous species. A large amount of experimental work has been devoted to an investigation of CN emission. However, up to now the plasma chemistry of CN radicals and processes leading to the excitation of CN electronic states are still poorly understood. The results of experimental measurements and numerical simulations are compared in order to establish the role of various channels of CN creation in the ground and excited states.
“…CO(v) significantly grows after oxygen is added (see e.g. [25,52,53] and references there). As that is not the case, one may deduce that (R13) is not a major channel of CN(B) production.…”
Section: Concentrations Of Cn Molecule In the Excited B 2 R Statementioning
The emission by electronically excited CN molecules is a prominent feature in the spectrum of active nitrogen containing traces of carbonaceous species. A large amount of experimental work has been devoted to an investigation of CN emission. However, up to now the plasma chemistry of CN radicals and processes leading to the excitation of CN electronic states are still poorly understood. The results of experimental measurements and numerical simulations are compared in order to establish the role of various channels of CN creation in the ground and excited states.
“…The influence of asymmetric intermolecular VV exchange (2) CO(V) + N 2 (0) ⇔ CО(V-2) + N 2 (1) + ∆E VJ ( 2 ) on G peak of a pulsed first overtone CO laser operating on ro-vibrational transitions V+2→V P(J) for V=34÷36 was also observed in [15]. Addition of N 2 molecules into gas mixture СО:Не resulted in more efficient depopulation of vibrational levels with V>37 and a decrease of G peak on ro-vibrational transitions of vibrational band 38→36 and enhancement G peak on vibrational band with V=34, respectively.…”
Section: Ssg Time Behavior For Gas Mixture Co:нe:о 2 =1:4:xmentioning
confidence: 99%
“…It was found in earlier studies [1][2][3] of self-sustained DC discharge CO laser that small additive of oxygen (up to 10 % of CO concentration) plays positive role in laser active medium (AM). A cause of such influence is connected with sufficient change of electric discharge characteristics [4], plasma structure [3,[5][6][7] and vibrational distribution function (VDF) of CO molecules [7,8] even at small addition of oxygen.…”
Temporal behavior of small signal gain in pulsed CO laser amplifier operating with oxygen rich gas mixtures CO:He:O 2 and CO:N 2 :O 2 was experimentally studied. The rich content of oxygen in helium mixture (CO:He:O 2 =1:4:2) resulted in ~8-fold increase of the maximum gain on low vibrational transitions (10→9) and strong absorption on high ones (21→20). A high efficient pulsed CO laser operating with gas mixture in which oxygen substituted for nitrogen was launched.
“…In addition, the interesting effects of gas additives on laser gain and wavelength in CO suggests that the plasma properties are being altered rather than a direct effect via molecular en-rgy transfer processes. 9 ) Since a shift in available laser wavelength toward / (where Q o is some arbitrary constant chosen to make the numbers 6 and n more manageable, we used Q =10~1 6 cm 2 ) we obtain Equations (4) and (5) are simultaneous first order differential equations for the distribution function and the inelastic collision integral. We solve these numerically using a fourth order Runge-Kutta integration scheme.…”
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